An existing Office 365 User can be set as Site collection administrator using cmdlet SET-SPOUser.
Following are the parameters.
Site
Site URL, where the user needs to be as site collection administrator.
LoginName
Login Name of User.
IsSiteCollectionAdmin
Boolean, try or false, true for setting as administrator, while false for removing a user as administrator.
Syntax
Following are the parameters.
Site
Site URL, where the user needs to be as site collection administrator.
LoginName
Login Name of User.
IsSiteCollectionAdmin
Boolean, try or false, true for setting as administrator, while false for removing a user as administrator.
Syntax
Set-SPOUser -Site <siteURL> -LoginName <UserLogin> -IsSiteCollectionAdmin <true/false>
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